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Insight into the mechanism of an iron dioxygenase by resolution of steps following the Fe(IV)═O species

Iron oxygenases generate elusive transient oxygen species to catalyze substrate oxygenation in a wide range of metabolic processes. Here we resolve the reaction sequence and structures of such intermediates for the archetypal non-heme Fe(II) and α-ketoglutarate-dependent dioxygenase TauD. Time-resol...

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Detalhes bibliográficos
Main Authors: Grzyska, Piotr K., Appelman, Evan H., Hausinger, Robert P., Proshlyakov, Denis A.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2840172/
https://ncbi.nlm.nih.gov/pubmed/20147623
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.0911565107
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