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Bifunctional Asymmetric Catalysis: Amplification of Brønsted Basicity Can Orthogonally Increase the Reactivity of a Chiral Brønsted Acid

[Image: see text] The reactivity of a series of symmetrical chiral Brønsted acids (polar ionic hydrogen bond donors) follows the counterintuitive trend wherein the more Brønsted basic member is a more effective catalyst for the aza-Henry (nitro-Mannich) reaction. This new design element leads to a s...

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Detalhes bibliográficos
Main Authors: Davis, Tyler A., Wilt, Jeremy C., Johnston, Jeffrey N.
Formato: Artigo
Idioma:Inglês
Publicado em: 2010
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2838452/
https://ncbi.nlm.nih.gov/pubmed/20151644
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja908814h
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