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Evolution of the Total Synthesis of (-)-Okilactomycin Exploiting a Tandem Oxy-Cope Rearrangement/Oxidation, the Petasis-Ferrier Union/Rearrangement and Ring Closing Metathesis

An effective, asymmetric total synthesis of the antitumor antibiotic (-)-okilactomycin (1) and assignment of the absolute configuration, has been achieved exploiting a convergent strategy. Highlights of the synthesis include: a diastereoselective oxy-Cope rearrangement/oxidation sequence to install...

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Detalhes bibliográficos
Main Authors: Smith, Amos B., Bosanac, Todd, Basu, Kallol
Formato: Artigo
Idioma:Inglês
Publicado em: 2009
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2697663/
https://ncbi.nlm.nih.gov/pubmed/19170499
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ja8084669
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