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Concise syntheses of enantiomerically pure protected 4-hydroxypyroglutamic acid and 4-hydroxyproline from a nitroso-cyclopentadiene cycloadduct

O-TBS-protected methyl trans-4-hydroxypyroglutamate and methyl trans-4-hydroxyproline ester were synthesized from nitroso-cyclopentadiene Diels-Alder cycloadducts. Enzymatic resolution of the key intermediate, 4-amino-cyclopent-2-enol, provides access to both L- and D- amino acids.

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Bibliographic Details
Main Authors: Huang, Weiqiang, Miller, Marvin J.
Format: Artigo
Language:Inglês
Published: 2008
Subjects:
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC2662620/
https://ncbi.nlm.nih.gov/pubmed/20011098
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tetasy.2008.12.013
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