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Multiple chirality transfers in the enantioselective synthesis of 11-O-debenzoyltashironin. Chiroptical analysis of the key cascade

The mechanism of the cascade oxidative dearomatization-transannular Diels Alder was investigated in the context of an asymmetric route to (−)-11-O-debenzoyltashironin. Although the oxidative dearomatization provides two acetal intermediates, the transannular Diels-Alder proceeds spontaneously from o...

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Detalhes bibliográficos
Main Authors: Polara, Alessandra, Cook, Silas P., Danishefsky, Samuel J.
Formato: Artigo
Idioma:Inglês
Publicado em: 2008
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2598418/
https://ncbi.nlm.nih.gov/pubmed/19812682
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1016/j.tetlet.2008.07.139
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