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Synthesis of (+)-Sch 642305 by a Biomimetic Transannular Michael Reaction

[Image: see text] The synthesis of (+)-Sch 642305 (1) has been completed in 17 steps in 1.6% overall yield. Transannular Michael reaction of 2b with NaH in THF provided cyclohexenone 23 stereospecifically. Heating 23 in TFA/CDCl(3) provided a 3:1 equilibrium mixture of 23 and 25, which were hydrolyz...

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Autors principals: Snider, Barry B., Zhou, Jingye
Format: Artigo
Idioma:Inglês
Publicat: 2006
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC2543932/
https://ncbi.nlm.nih.gov/pubmed/16562872
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol052948+
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