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Biomimetic Synthesis of the Tetracyclic Core of Berkelic Acid

[Image: see text] Acid catalyzed condensation of 2,6-dihydroxybenzoic acid 3 with ketal aldehyde 14 in methanol at 25 °C, followed by CH(2)N(2) esterification gave a 4:1:4:1 mixture of diastereomers 15b-18b in 60% yield. Equilibration of this mixture with TFA in CDCl(3) provided tetracycle 15b (83%...

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Detalhes bibliográficos
Main Authors: Zhou, Jingye, Snider, Barry B.
Formato: Artigo
Idioma:Inglês
Publicado em: 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2527759/
https://ncbi.nlm.nih.gov/pubmed/17465557
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol0704338
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