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Hydrogen Bonding Catalysis Operates by Charge Stabilization in Highly Polar Diels–Alder Reactions

The alcohol-catalyzed Diels-Alder reactions of acrolein and benzaldehyde with Rawal’s diene were evaluated with density functional theory (B3LYP/6-31G(d)). Several potential modes of catalysis with two methanol molecules were used to model catalysis by TADDOLs. In agreement with crystallographic dat...

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Detalhes bibliográficos
Main Authors: Gordillo, Ruth, Dudding, Travis, Anderson, Christopher D., Houk, K. N.
Formato: Artigo
Idioma:Inglês
Publicado em: 2007
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC2531143/
https://ncbi.nlm.nih.gov/pubmed/17249797
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/ol0629925
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