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Isotope Effects and the Mechanism of Epoxidation of Cyclohexenone with tert-Butyl Hydroperoxide

The mechanism of the epoxidation of 2-cyclohexen-1-one with tert-butyl hydroperoxide mediated by DBU was studied by a combination of experimental kinetic isotope effects and theoretical calculations. A large (12)C/(13)C (k(12(C))/k(13(C))) isotope effect of ≈1.032 was observed at the C(3) (β) positi...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Hauptverfasser: Christian, Chad F., Takeya, Tetsuya, Szymanski, Michael J., Singleton, Daniel A.
Format: Artigo
Sprache:Inglês
Veröffentlicht: 2007
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC2465813/
https://ncbi.nlm.nih.gov/pubmed/17608437
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jo070777b
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