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Synthesis of the polyketide section of seragamide A and related cyclodepsipeptides via Negishi cross coupling

The synthesis of the polyketide section present in the potently cytotoxic marine cyclodepsipeptide jasplakinolide and related natural products, geodiamolides and seragamides, is reported. The key step is a Negishi cross coupling of (R)-(3-methoxy-2-methyl-3-oxopropyl)zinc(II) bromide and an (E)-iodo...

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Principais autores: Jan Hendrik Lang, Thomas Lindel
Format: Artigo
Sprog:Inglês
Udgivet: Beilstein-Institut 2019-02-01
Serier:Beilstein Journal of Organic Chemistry
Fag:
jasplakinolide
marine natural products
Negishi coupling
polyketides
stereoselective synthesis
Online adgang:https://doi.org/10.3762/bjoc.15.53
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