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Generation of Masked Ti(II) Intermediates from Ti(IV) Amides via β-H Abstraction or Alkyne Deprotonation: An Example of Ti-Catalyzed Nitrene-Coupled Transfer Hydrogenation

Simple Ti amide complexes are shown to act as sources for masked Ti(II) intermediates via several pathways, as demonstrated through the investigation of a unique Ti-catalyzed nitrene-coupled transfer hydrogenation of 3-hexyne. This reaction proceeds through reduction of azobenzene by a masked Ti(II)...

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Detalhes bibliográficos
Publicado no:Organometallics
Main Authors: Pearce, Adam J., Cheng, Yukun, Dunscomb, Rachel J., Tonks, Ian A.
Formato: Artigo
Idioma:Inglês
Publicado em: 2020
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8315702/
https://ncbi.nlm.nih.gov/pubmed/34321708
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.organomet.0c00577
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