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Unveiling the spatial distribution of molecular coherences at conical intersections by covariance X-ray diffraction signals

The outcomes and timescales of molecular nonadiabatic dynamics are decisively impacted by the quantum coherences generated at localized molecular regions. In time-resolved X-ray diffraction imaging, these coherences create distinct signatures via inelastic photon scattering, but they are buried unde...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Main Authors: Cavaletto, Stefano M., Keefer, Daniel, Rouxel, Jérémy R., Aleotti, Flavia, Segatta, Francesco, Garavelli, Marco, Mukamel, Shaul
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC8179141/
https://ncbi.nlm.nih.gov/pubmed/34050030
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.2105046118
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