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Signatures of electronic and nuclear coherences in ultrafast molecular x-ray and electron diffraction

Femtosecond x-ray and electron diffraction hold promise to image the evolving structures of single molecules. We present a unified quantum-electrodynamical formulation of diffraction signals, based on the exact many-body nuclear + electronic wavefunction that can be extracted from quantum chemistry...

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Detalhes bibliográficos
Publicado no:Struct Dyn
Main Authors: Rouxel, Jérémy R., Keefer, Daniel, Mukamel, Shaul
Formato: Artigo
Idioma:Inglês
Publicado em: American Crystallographic Association 2021
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7803382/
https://ncbi.nlm.nih.gov/pubmed/33457447
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1063/4.0000043
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