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How the Lewis Base F(–) Catalyzes the 1,3-Dipolar Cycloaddition between Carbon Dioxide and Nitrilimines
[Image: see text] The mechanism of the Lewis base F(–) catalyzed 1,3-dipolar cycloaddition between CO(2) and nitrilimines is interrogated using DFT calculations. F(–) activates the nitrilimine, not CO(2) as proposed in the literature, and imparts a significant rate enhancement for the cycloaddition....
Guardat en:
| Publicat a: | J Org Chem |
|---|---|
| Autors principals: | , , , |
| Format: | Artigo |
| Idioma: | Inglês |
| Publicat: |
American Chemical
Society
2021
|
| Accés en línia: | https://ncbi.nlm.nih.gov/pmc/articles/PMC8023701/ https://ncbi.nlm.nih.gov/pubmed/33577314 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.joc.0c02963 |
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