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Ferric Heme Superoxide Reductive Transformations to Ferric Heme (Hydro)Peroxide Species: Spectroscopic Characterization and Thermodynamic Implications for H-atom Transfer (HAT)
A new end-on low-spin ferric heme peroxide, [(P(Im))Fe(III)─(O(2)(2−))](−) (P(Im)-P), and subsequently formed hydroperoxide species, [(P(Im))Fe(III)─(OOH)] (P(Im)-HP) are generated utilizing the iron-porphyrinate P(Im) with its tethered axial base imidazolyl group. Measured thermodynamic parameters,...
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| Publicado no: | Angew Chem Int Ed Engl |
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| Main Authors: | , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2021
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC7920932/ https://ncbi.nlm.nih.gov/pubmed/33348450 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202013791 |
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