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On the Structure of Intermediates in Enyne Gold(I)‐Catalyzed Cyclizations: Formation of trans‐Fused Bicyclo[5.1.0]octanes as a Case Study

The nature of cyclopropyl gold(I) carbene‐type intermediates has been reexamined as part of a mechanistic study on the formation of cis‐ or trans‐fused bicyclo[5.1.0]octanes in a gold(I)‐catalyzed cascade reaction. Benchmark of DFT methods together with QTAIM theory and NBO analysis confirms the for...

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Publicat a:Chemistry
Autors principals: Escofet, Imma, Armengol‐Relats, Helena, Bruss, Hanna, Besora, Maria, Echavarren, Antonio M.
Format: Artigo
Idioma:Inglês
Publicat: John Wiley and Sons Inc. 2020
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Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC7756441/
https://ncbi.nlm.nih.gov/pubmed/33155306
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/chem.202004237
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