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Unraveling the Mechanism of the Ir(III)‐Catalyzed Regiospecific Synthesis of α‐Chlorocarbonyl Compounds from Allylic Alcohols

We have used experimental studies and DFT calculations to investigate the Ir(III)‐catalyzed isomerization of allylic alcohols into carbonyl compounds, and the regiospecific isomerization–chlorination of allylic alcohols into α‐chlorinated carbonyl compounds. The mechanism involves a hydride eliminat...

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Detalhes bibliográficos
Publicado no:Chemistry
Main Authors: Li, Man, Sanz‐Marco, Amparo, Martinez‐Erro, Samuel, García‐Vázquez, Víctor, Mai, Binh Khanh, Fernández‐Gallardo, Jacob, Himo, Fahmi, Martín‐Matute, Belén
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2020
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Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7756427/
https://ncbi.nlm.nih.gov/pubmed/32757212
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/chem.202002845
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