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Chemically triggered crosslinking with bioorthogonal cyclopropenones

We report a proximity-driven crosslinking strategy featuring bioorthogonal cyclopropenones. These motifs react with phosphines to form electrophilic ketene-ylides. Such intermediates can be trapped by neighboring proteins to form covalent adducts. Successful crosslinking was achieved using a model s...

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Publicat a:Chem Commun (Camb)
Autors principals: Row, R. David, Nguyen, Sean S., Ferreira, Andrew J., Prescher, Jennifer A.
Format: Artigo
Idioma:Inglês
Publicat: 2020
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC7501174/
https://ncbi.nlm.nih.gov/pubmed/32808608
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/d0cc04600k
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