Interplay of Electronic and Steric Effects to Yield Low‐Temperature CO Oxidation at Metal Single Sites in Defect‐Engineered HKUST‐1

In contrast to catalytically active metal single atoms deposited on oxide nanoparticles, the crystalline nature of metal‐organic frameworks (MOFs) allows for a thorough characterization of reaction mechanisms. Using defect‐free HKUST‐1 MOF thin films, we demonstrate that Cu(+)/Cu(2+) dimer defects,...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Wang, Weijia, Sharapa, Dmitry I., Chandresh, Abhinav, Nefedov, Alexei, Heißler, Stefan, Heinke, Lars, Studt, Felix, Wang, Yuemin, Wöll, Christof
Formato: Artigo
Idioma:Inglês
Publicado em: John Wiley and Sons Inc. 2020
Assuntos:
Communications
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7318571/
https://ncbi.nlm.nih.gov/pubmed/32196128
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202000385
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