Interplay of Electronic and Steric Effects to Yield Low‐Temperature CO Oxidation at Metal Single Sites in Defect‐Engineered HKUST‐1

In contrast to catalytically active metal single atoms deposited on oxide nanoparticles, the crystalline nature of metal‐organic frameworks (MOFs) allows for a thorough characterization of reaction mechanisms. Using defect‐free HKUST‐1 MOF thin films, we demonstrate that Cu(+)/Cu(2+) dimer defects,...

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Tallennettuna:
Bibliografiset tiedot
Julkaisussa:Angew Chem Int Ed Engl
Päätekijät: Wang, Weijia, Sharapa, Dmitry I., Chandresh, Abhinav, Nefedov, Alexei, Heißler, Stefan, Heinke, Lars, Studt, Felix, Wang, Yuemin, Wöll, Christof
Aineistotyyppi: Artigo
Kieli:Inglês
Julkaistu: John Wiley and Sons Inc. 2020
Aiheet:
Communications
Linkit:https://ncbi.nlm.nih.gov/pmc/articles/PMC7318571/
https://ncbi.nlm.nih.gov/pubmed/32196128
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.202000385
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