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Vicinal, Double C-H Functionalization of Alcohols via an Imidate Radical-Polar Crossover Cascade

A double functionalization of vicinal sp(3) C-H bonds has been developed, wherein a β amine and γ iodide are incorporated onto an aliphatic alcohol in a single operation. This approach is enabled by an imidate radical chaperone, which selectively affords a transient β alkene that is amino-iodinated...

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Publicado en:J Am Chem Soc
Main Authors: Prusinowski, Allen F., Twumasi, Raymond K., Wappes, Ethan A., Nagib, David A.
Formato: Artigo
Idioma:Inglês
Publicado: 2020
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC7299201/
https://ncbi.nlm.nih.gov/pubmed/32141741
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.0c01318
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