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Control of stereoselectivity in diverse hapalindole metabolites is mediated by cofactor induced combinatorial pairing of Stig cyclases

The stereospecific polycyclic core formation of hapalindoles and fischerindoles is controlled by the Stig cyclases through a three-step cascade involving Cope rearrangement, 6-exo-trig cyclization and a final electrophilic aromatic substitution. Here we report a comprehensive study of all currently...

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Bibliografske podrobnosti
izdano v:Angew Chem Int Ed Engl
Main Authors: Li, Shasha, Newmister, Sean A., Lowell, Andrew N., Zi, Jiachen, Chappell, Callie R., Yu, Fengan, Hohlman, Robert M., Orjala, Jimmy, Williams, Robert M., Sherman, David H.
Format: Artigo
Jezik:Inglês
Izdano: 2020
Teme:
Online dostop:https://ncbi.nlm.nih.gov/pmc/articles/PMC7274885/
https://ncbi.nlm.nih.gov/pubmed/32052896
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201913686
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