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Synthesis of Pyridylimido Complexes of Tantalum and Niobium by Reductive Cleavage of the N=N Bond of 2,2′-Azopyridine: Precursors for Early–Late Heterobimetallic Complexes

We report the syntheses of 2-pyridylimido complexes of tantalum and niobium by N=N bond cleavage of 2,2′-azopyridine. Reaction of MCl(5) (M = Ta and Nb) with 2,2′-azopyridine in the presence of 0.5 equiv of 1-methyl-3,6-bis(trimethylsilyl)-1,4-cyclohexadiene (abbreviated Si-Me-CHD) afforded a dark r...

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Detalhes bibliográficos
Publicado no:Inorg Chem
Main Authors: Kawakita, Kento, Kakiuchi, Yuya, Beaumier, Evan P., Tonks, Ian A., Tsurugi, Hayato, Mashima, Kazushi
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC7017918/
https://ncbi.nlm.nih.gov/pubmed/31553585
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.inorgchem.9b02043
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