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The Critical Role of Reductive Steps in the Nickel‐Catalyzed Hydrogenolysis and Hydrolysis of Aryl Ether C−O Bonds

The hydrogenolysis of the aromatic C−O bond in aryl ethers catalyzed by Ni was studied in decalin and water. Observations of a significant kinetic isotope effect (k (H)/k (D)=5.7) for the reactions of diphenyl ether under H(2) and D(2) atmosphere and a positive dependence of the rate on H(2) chemica...

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Bibliografiske detaljer
Udgivet i:Angew Chem Int Ed Engl
Main Authors: Wang, Meng, Zhao, Yuntao, Mei, Donghai, Bullock, R. Morris, Gutiérrez, Oliver Y., Camaioni, Donald M., Lercher, Johannes A.
Format: Artigo
Sprog:Inglês
Udgivet: John Wiley and Sons Inc. 2019
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC7003888/
https://ncbi.nlm.nih.gov/pubmed/31512341
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201909551
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