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Regulating the Basicity of Metal–Oxido Complexes with a Single Hydrogen Bond and its Effect on C–H Bond Cleavage

The functionalization of C–H bonds is an essential reaction in biology and chemistry. Metalloenzymes that often exhibit this type of reactivity contain metal-oxido intermediates which are directly involved the initial cleavage of the C–H bonds. Regulation of the cleavage process is achieved, in part...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Barman, Suman K., Jones, Jason R., Sun, Chen, Hill, Ethan A., Ziller, Joseph W., Borovik, A. S.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6776423/
https://ncbi.nlm.nih.gov/pubmed/31274298
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b03688
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