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Hemilabile Benzyl Ether Enables γ-C(sp(3))–H Carbonylation and Olefination of Alcohols

Pd-catalyzed C(sp(3))–H activation of alcohol typically shows β-selectivity due to the required distance between the chelating atom in the attached directing group and the targeted C–H bonds. Herein we report the design of hemilabile directing group, which exploit the chelation of a readily removabl...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Tanaka, Keita, Ewing, William R., Yu, Jin-Quan
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6776245/
https://ncbi.nlm.nih.gov/pubmed/31519108
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b08238
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