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Transition state analysis of an enantioselective Michael addition by a bifunctional thiourea organocatalyst

The mechanism of the enantioselective Michael addition of diethyl malonate to trans-β-nitrostyrene catalyzed by a tertiary amine thiourea organocatalyst is explored using experimental (13)C kinetic isotope effects and density functional theory calculations. Large primary (13)C KIEs on the bond-formi...

Disgrifiad llawn

Wedi'i Gadw mewn:
Manylion Llyfryddiaeth
Cyhoeddwyd yn:Org Biomol Chem
Prif Awduron: Izzo, Joseph A., Myshchuk, Yaroslaw, Hirschi, Jennifer S., Vetticatt, Mathew J.
Fformat: Artigo
Iaith:Inglês
Cyhoeddwyd: 2019
Pynciau:
Mynediad Ar-lein:https://ncbi.nlm.nih.gov/pmc/articles/PMC6774437/
https://ncbi.nlm.nih.gov/pubmed/30942247
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9ob00072k
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