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Spectroscopic Characterization of an Eight-Iron Nitrogenase Cofactor Precursor That Lacks the “9(th) Sulfur”

Nitrogenase catalyzes the reduction of N(2) to NH(4)(+) at its cofactor site. Designated the M-cluster, this [MoFe(7)S(9)C(R-homocitrate)] cofactor is synthesized via transformation of a [Fe(4)S(4)] cluster pair into an [Fe(8)S(9)C] precursor (designated the L-cluster) prior to insertion of Mo and h...

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Detalhes bibliográficos
Publicado no:Angew Chem Int Ed Engl
Main Authors: Jasniewski, Andrew J., Wilcoxen, Jarett, Tanifuji, Kazuki, Hedman, Britt, Hodgson, Keith O., Britt, R. David, Hu, Yilin, Ribbe, Markus W.
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6764854/
https://ncbi.nlm.nih.gov/pubmed/31411369
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1002/anie.201907593
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