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Tracing the ‘9(th) Sulfur’ of the Nitrogenase Cofactor via a Semi-Synthetic Approach
The M-cluster is the [(homocitrate)MoFe(7)S(9)C] active site of nitrogenase that is derived from an 8Fe core assembled via coupling and rearrangement of two [Fe(4)S(4)] clusters concomitant with the insertion of an interstitial carbon and a ‘9(th) sulfur’. Combining synthetic [Fe(4)S(4)] clusters wi...
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| Publicado en: | Nat Chem |
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| Autores principales: | , , , , , , |
| Formato: | Artigo |
| Lenguaje: | Inglês |
| Publicado: |
2018
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| Materias: | |
| Acceso en línea: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5910187/ https://ncbi.nlm.nih.gov/pubmed/29662207 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41557-018-0029-4 |
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