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Engineering opposite electronic polarization of singlet and triplet states increases the yield of high-energy photoproducts

Efficient photosynthetic energy conversion requires quantitative, light-driven formation of high-energy, charge-separated states. However, energies of high-lying excited states are rarely extracted, in part because the congested density of states in the excited-state manifold leads to rapid deactiva...

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Detalhes bibliográficos
Publicado no:Proc Natl Acad Sci U S A
Main Authors: Polizzi, Nicholas F., Jiang, Ting, Beratan, David N., Therien, Michael J.
Formato: Artigo
Idioma:Inglês
Publicado em: National Academy of Sciences 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6642396/
https://ncbi.nlm.nih.gov/pubmed/31182609
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1073/pnas.1901752116
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