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Tuning the Geometric and Electronic Structure of Synthetic High-Valent Heme Iron(IV)-Oxo Models in the Presence of a Lewis Acid and Various Axial Ligands
High-valent ferryl species (e.g., (Por)Fe(IV)=O, Cmpd-II) are observed or proposed key oxidizing intermediates in the catalytic cycles of heme-containing enzymes (P-450s, peroxidases, catalases, and cytochrome c oxidase) involved in biological respiration and oxidative metabolism. Herein, various ax...
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| Publicado no: | J Am Chem Soc |
|---|---|
| Main Authors: | , , , , , , , , |
| Formato: | Artigo |
| Idioma: | Inglês |
| Publicado em: |
2019
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| Assuntos: | |
| Acesso em linha: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6611672/ https://ncbi.nlm.nih.gov/pubmed/30860832 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.9b00795 |
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