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Enantioselective Conia-Ene-Type Cyclizations of Alkynyl Ketones through Cooperative Action of B(C(6)F(5))(3), N-Alkylamine and a Zn-Based Catalyst

An efficient and highly enantioselective Conia-ene-type process has been developed. Reactions are catalyzed by a combination of B(C(6)F(5))(3), an N-alkylamine and a BOX–ZnI(2) complex. Specifically, through cooperative action of B(C(6)F(5))(3) and amine, ketones with poorly acidic α-C–H bonds can b...

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Detalhes bibliográficos
Publicado no:J Am Chem Soc
Main Authors: Cao, Min, Yesilcimen, Ahmet, Wasa, Masayuki
Formato: Artigo
Idioma:Inglês
Publicado em: 2019
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6595478/
https://ncbi.nlm.nih.gov/pubmed/30786707
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b13757
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