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One metal is enough: a nickel complex reduces nitrate anions to nitrogen gas

A stepwise reduction sequence from nitrate to dinitrogen gas at a single nickel center was discovered. A PNP nickel scaffold (PNP(–) = N[2-P(i)Pr(2)-4-Me-C(6)H(3)](2)) emerged as a universal platform for the deoxygenation of NO(x) substrates. In these reactions carbon monoxide acts as the oxygen acc...

Ausführliche Beschreibung

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Bibliographische Detailangaben
Veröffentlicht in:Chem Sci
Hauptverfasser: Gwak, Jinseong, Ahn, Seihwan, Baik, Mu-Hyun, Lee, Yunho
Format: Artigo
Sprache:Inglês
Veröffentlicht: Royal Society of Chemistry 2019
Schlagworte:
Online Zugang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6510316/
https://ncbi.nlm.nih.gov/pubmed/31160953
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc00717b
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