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Radical Hydroarylation of Functionalized Olefins and Mechanistic Investigation of Photocatalytic Pyridyl Radical Reactions

We report the photoredox alkylation of halopyridines using functionalized alkene and alkyne building blocks. Selective single-electron reduction of the halogenated pyridines provides the corresponding heteroaryl radicals, which undergo anti-Markovnikov addition to the alkene substrates. The system i...

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Publicat a:J Am Chem Soc
Autors principals: Seath, Ciaran P., Vogt, David B., Xu, Zihao, Boyington, Allyson J., Jui, Nathan T.
Format: Artigo
Idioma:Inglês
Publicat: 2018
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC6495588/
https://ncbi.nlm.nih.gov/pubmed/30354095
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.8b10238
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