Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study

(99)Tc is one of the most problematic fission products in the nuclear fuel cycle owing to its large inventory in used nuclear fuel, long half-life, potential radiation hazard, high environmental mobility of its major species (99)TcO(4)(–), and its redox-active nature. Ideally, (99)TcO(4)(–) should b...

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Bibliographic Details
Published in:Chem Sci
Main Authors: He, Linwei, Liu, Shengtang, Chen, Long, Dai, Xing, Li, Jie, Zhang, Mingxing, Ma, Fuyin, Zhang, Chao, Yang, Zaixing, Zhou, Ruhong, Chai, Zhifang, Wang, Shuao
Format: Artigo
Language:Inglês
Published: Royal Society of Chemistry 2019
Subjects:
Chemistry
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC6471554/
https://ncbi.nlm.nih.gov/pubmed/31057756
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc00172g
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