Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study

(99)Tc is one of the most problematic fission products in the nuclear fuel cycle owing to its large inventory in used nuclear fuel, long half-life, potential radiation hazard, high environmental mobility of its major species (99)TcO(4)(–), and its redox-active nature. Ideally, (99)TcO(4)(–) should b...

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Bibliografiske detaljer
Udgivet i:	Chem Sci
Main Authors:	He, Linwei, Liu, Shengtang, Chen, Long, Dai, Xing, Li, Jie, Zhang, Mingxing, Ma, Fuyin, Zhang, Chao, Yang, Zaixing, Zhou, Ruhong, Chai, Zhifang, Wang, Shuao
Format:	Artigo
Sprog:	Inglês
Udgivet:	Royal Society of Chemistry 2019
Fag:	Chemistry
Online adgang:	https://ncbi.nlm.nih.gov/pmc/articles/PMC6471554/ https://ncbi.nlm.nih.gov/pubmed/31057756 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c9sc00172g
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Mechanism unravelling for ultrafast and selective (99)TcO(4)(–) uptake by a radiation-resistant cationic covalent organic framework: a combined radiological experiment and molecular dynamics simulation study

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