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Enantioselective synthesis of gem-disubstituted N-Boc diazaheterocycles via decarboxylative asymmetric allylic alkylation

An enantioselective synthesis of diverse N4-Boc-protected α,α-disubstituted piperazin-2-ones using the palladium-catalyzed decarboxylative allylic alkylation reaction has been achieved. Using a chiral Pd-catalyst derived from an electron deficient PHOX ligand, chiral piperazinones are synthesized in...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Sun, Alexander W., Hess, Stephan N., Stoltz, Brian M.
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2018
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6345351/
https://ncbi.nlm.nih.gov/pubmed/30774872
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c8sc03967d
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