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pH effects on the electrochemical reduction of CO((2)) towards C(2) products on stepped copper
We present a microkinetic model for CO((2)) reduction (CO((2))R) on Cu(211) towards C(2) products, based on energetics estimated from an explicit solvent model. We show that the differences in both Tafel slopes and pH dependence for C(1) vs C(2) activity arise from differences in their multi-step me...
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| 出版年: | Nat Commun |
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| 主要な著者: | , , , , , , , , , , , , , |
| フォーマット: | Artigo |
| 言語: | Inglês |
| 出版事項: |
Nature Publishing Group UK
2019
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| 主題: | |
| オンライン･アクセス: | https://ncbi.nlm.nih.gov/pmc/articles/PMC6318338/ https://ncbi.nlm.nih.gov/pubmed/30604776 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41467-018-07970-9 |
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