pH effects on the electrochemical reduction of CO((2)) towards C(2) products on stepped copper

We present a microkinetic model for CO((2)) reduction (CO((2))R) on Cu(211) towards C(2) products, based on energetics estimated from an explicit solvent model. We show that the differences in both Tafel slopes and pH dependence for C(1) vs C(2) activity arise from differences in their multi-step me...

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Detalhes bibliográficos
Publicado no:Nat Commun
Main Authors: Liu, Xinyan, Schlexer, Philomena, Xiao, Jianping, Ji, Yongfei, Wang, Lei, Sandberg, Robert B., Tang, Michael, Brown, Kristopher S., Peng, Hongjie, Ringe, Stefan, Hahn, Christopher, Jaramillo, Thomas F., Nørskov, Jens K., Chan, Karen
Formato: Artigo
Idioma:Inglês
Publicado em: Nature Publishing Group UK 2019
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Article
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC6318338/
https://ncbi.nlm.nih.gov/pubmed/30604776
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1038/s41467-018-07970-9
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