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Tyrosine-coordinated P-cluster in G. diazotrophicus nitrogenase: Evidence for the importance of O-based ligands in conformationally gated electron transfer

The P-cluster is a unique iron-sulfur center that likely functions as a dynamic electron (e(−)) relay site between the Fe-protein and the catalytic FeMo-cofactor in nitrogenase. The P-cluster has been shown to undergo large conformational changes upon 2-e(−) oxidation which entail the coordination o...

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Udgivet i:J Am Chem Soc
Main Authors: Owens, Cedric P., Katz, Faith E. H., Carter, Cole H., Oswald, Victoria F., Tezcan, F. Akif
Format: Artigo
Sprog:Inglês
Udgivet: 2016
Fag:
Online adgang:https://ncbi.nlm.nih.gov/pmc/articles/PMC6129449/
https://ncbi.nlm.nih.gov/pubmed/27487256
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b06783
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