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Direct catalytic enantioselective amination of ketones for the formation of tri- and tetrasubstituted stereocenters

Herein, we report a Zn–ProPhenol catalyzed direct asymmetric amination reaction of unactivated aryl and vinyl ketones using di-tert-butyl azodicarboxylate as a cheap and practical electrophilic nitrogen source. Importantly, this methodology works with both α-branched and unbranched ketones for the c...

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Publicado en:Chem Sci
Main Authors: Trost, B. M., Tracy, J. S., Saget, T.
Formato: Artigo
Idioma:Inglês
Publicado: Royal Society of Chemistry 2018
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Acceso en liña:https://ncbi.nlm.nih.gov/pmc/articles/PMC5897889/
https://ncbi.nlm.nih.gov/pubmed/29719678
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c8sc00147b
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