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Direct Comparison of C–H Bond Amination Efficacy through Manipulation of Nitrogen-Valence Centered Redox: Imido versus Iminyl
Reduction of previously reported iminyl radical ((Ar)L)FeCl((•)N(C(6)H(4)-p-(t)Bu)) (2) with potassium graphite furnished the corresponding high-spin (S = (5)/(2)) imido ((Ar)L)Fe(N(C(6)H(4)-p-(t)Bu)) (3) ((Ar)L = 5-mesityl-1,9-(2,4,6-Ph(3)C(6)H(2))dipyrrin). Oxidation of the three-coordinate imido...
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| 出版年: | J Am Chem Soc |
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| 主要な著者: | , , , , , , |
| フォーマット: | Artigo |
| 言語: | Inglês |
| 出版事項: |
2017
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| 主題: | |
| オンライン･アクセス: | https://ncbi.nlm.nih.gov/pmc/articles/PMC5821126/ https://ncbi.nlm.nih.gov/pubmed/28937756 https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.7b08714 |
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