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What is the trigger mechanism for the reversal of electron flow in oxygen-tolerant [NiFe] hydrogenases?

The [NiFe] hydrogenases use an electron transfer relay of three FeS clusters – proximal, medial and distal – to release the electrons from the principal reaction, H(2) → 2H(+) + 2e(–), that occurs at the Ni–Fe catalytic site. This site is normally inactivated by O(2), but the subclass of O(2)-tolera...

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Detalhes bibliográficos
Publicado no:Chem Sci
Autor principal: Dance, Ian
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2015
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5811149/
https://ncbi.nlm.nih.gov/pubmed/29560232
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c4sc03223c
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