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Dehydrogenation, disproportionation and transfer hydrogenation reactions of formic acid catalyzed by molybdenum hydride compounds

The cyclopentadienyl molybdenum hydride compounds, Cp(R)Mo(PMe(3))(3–x)(CO)(x)H (Cp(R) = Cp, Cp*; x = 0, 1, 2 or 3), are catalysts for the dehydrogenation of formic acid, with the most active catalysts having the composition Cp(R)Mo(PMe(3))(2)(CO)H. The mechanism of the catalytic cycle is proposed t...

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Bibliographic Details
Published in:Chem Sci
Main Authors: Neary, Michelle C., Parkin, Gerard
Format: Artigo
Language:Inglês
Published: Royal Society of Chemistry 2015
Subjects:
Online Access:https://ncbi.nlm.nih.gov/pmc/articles/PMC5649328/
https://ncbi.nlm.nih.gov/pubmed/29308136
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c4sc03128h
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