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A novel application of 2-silylated 1,3-dithiolanes for the synthesis of aryl/hetaryl-substituted ethenes and dibenzofulvenes

Trimethylsilyldiazomethane (TMS-CHN(2)) reacts readily with hetaryl thioketones to give sterically crowded 2-trimethylsilyl-4,4,5,5-tetrahetaryl-1,3-dithiolanes with complete regioselectivity at −75 °C as well as at rt. Thiofluorenone, a relatively stable and highly reactive aryl thioketone, yields...

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Detalhes bibliográficos
Publicado no:Beilstein J Org Chem
Main Authors: Mlostoń, Grzegorz, Pipiak, Paulina, Hamera-Fałdyga, Róża, Heimgartner, Heinz
Formato: Artigo
Idioma:Inglês
Publicado em: Beilstein-Institut 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5629374/
https://ncbi.nlm.nih.gov/pubmed/29062409
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.3762/bjoc.13.185
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