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A highly convergent synthesis of the C1–C31 polyol domain of amphidinol 3 featuring a TST-RCM reaction: confirmation of the revised relative stereochemistry

The concise enantioselective synthesis of the revised C1–C31 fragment of the polyketide amphidinol 3 was accomplished in 16 steps and 12.8% overall yield. Salient features of the strategy include chemoselective Weinreb amide coupling and concomitant CBS reduction for the preparation of the C1–C15 tr...

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Vydáno v:Chem Sci
Hlavní autoři: Grisin, Aleksandr, Evans, P. Andrew
Médium: Artigo
Jazyk:Inglês
Vydáno: Royal Society of Chemistry 2015
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On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC5507186/
https://ncbi.nlm.nih.gov/pubmed/28757956
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c5sc00814j
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