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Mechanistic study of the rhodium-catalyzed carboxylation of simple aromatic compounds with carbon dioxide

A detailed mechanism of the Rh(i)-catalyzed carboxylation of simple aromatic compounds via C–H bond activation was investigated. Kinetic studies with model compounds of the postulated key intermediates revealed that 14-electron complexes, RhMe(dcype) and RhPh(dcype), participated in the C–H bond act...

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Vydáno v:Chem Sci
Hlavní autoři: Suga, Takuya, Saitou, Takanobu, Takaya, Jun, Iwasawa, Nobuharu
Médium: Artigo
Jazyk:Inglês
Vydáno: Royal Society of Chemistry 2017
Témata:
On-line přístup:https://ncbi.nlm.nih.gov/pmc/articles/PMC5460598/
https://ncbi.nlm.nih.gov/pubmed/28616144
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc03838g
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