Probing Transient Valence Orbital Changes with Picosecond Valence-to-Core X-ray Emission Spectroscopy

[Image: see text] We probe the dynamics of valence electrons in photoexcited [Fe(terpy)(2)](2+) in solution to gain deeper insight into the Fe–ligand bond changes. We use hard X-ray emission spectroscopy (XES), which combines element specificity and high penetration with sensitivity to orbital struc...

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Detalhes bibliográficos
Publicado no:J Phys Chem C Nanomater Interfaces
Main Authors: March, Anne Marie, Assefa, Tadesse A., Boemer, Christina, Bressler, Christian, Britz, Alexander, Diez, Michael, Doumy, Gilles, Galler, Andreas, Harder, Manuel, Khakhulin, Dmitry, Németh, Zoltán, Pápai, Mátyás, Schulz, Sebastian, Southworth, Stephen H., Yavaş, Hasan, Young, Linda, Gawelda, Wojciech, Vankó, György
Formato: Artigo
Idioma:Inglês
Publicado em: American Chemical Society 2017
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5453616/
https://ncbi.nlm.nih.gov/pubmed/28580048
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/acs.jpcc.6b12940
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