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Predicting reaction coordinates in energy landscapes with diffusion anisotropy

We consider a range of model potentials with metastable states undergoing molecular dynamics coupled to a thermal bath in the high friction regime and consider how the optimal reaction coordinate depends on the diffusion anisotropy. For this we use our recently proposed method “spectral gap optimiza...

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Publicat a:J Chem Phys
Autors principals: Tiwary, Pratyush, Berne, B. J.
Format: Artigo
Idioma:Inglês
Publicat: AIP Publishing LLC 2017
Matèries:
Accés en línia:https://ncbi.nlm.nih.gov/pmc/articles/PMC5446309/
https://ncbi.nlm.nih.gov/pubmed/29055314
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1063/1.4983727
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