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Synthesis of Secondary Unsaturated Lactams via an Aza-Heck Reaction

The preparation of unsaturated secondary lactams via the palladium-catalyzed cyclization of O-phenyl hydroxamates onto a pendent alkene is reported. This method provides rapid access to a broad range of lactams that are widely useful building blocks in alkaloid synthesis. Mechanistic studies support...

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Pubblicato in:J Am Chem Soc
Autori principali: Shuler, Scott A., Yin, Guoyin, Krause, Sarah B., Vesper, Caroline M., Watson, Donald A.
Natura: Artigo
Lingua:Inglês
Pubblicazione: 2016
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Accesso online:https://ncbi.nlm.nih.gov/pmc/articles/PMC5395365/
https://ncbi.nlm.nih.gov/pubmed/27754648
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1021/jacs.6b08932
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