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Enantioselective allylic alkylation of stereodefined polysubstituted copper enolates as an entry to acyclic quaternary carbon stereocentres

A sequence of regio- and stereoselective carbometalation followed by oxidation of ynamides leads to stereodefined fully substituted enolates that subsequently react with various functionalized allyl bromide reagents to provide the expected products possessing an enantiomerically pure quaternary carb...

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Detalhes bibliográficos
Publicado no:Chem Sci
Main Authors: Nairoukh, Zackaria, Kumar, Gunda G. K. S. Narayana, Minko, Yury, Marek, Ilan
Formato: Artigo
Idioma:Inglês
Publicado em: Royal Society of Chemistry 2017
Assuntos:
Acesso em linha:https://ncbi.nlm.nih.gov/pmc/articles/PMC5358538/
https://ncbi.nlm.nih.gov/pubmed/28451210
https://ncbi.nlm.nih.govhttp://dx.doi.org/10.1039/c6sc03036j
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